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Fatty Acid Synthesis & Beta-Oxidation

Biochemistry · Lipids · lean revision notes

Fatty Acid Synthesis & Beta-Oxidation

Fatty acid metabolism is a perennial NEET PG high-scorer because it links enzymology, compartmentalisation, vitamin cofactors, regulation and inborn errors in a single, tightly examined web. Mastering the two opposing pathways — cytosolic synthesis (lipogenesis) and mitochondrial β-oxidation — together with the carnitine shuttle and MCAD deficiency, reliably fetches 2–3 marks every cycle.

Big-picture orientation

The two pathways are deliberately separated so they never run simultaneously (futile cycling is prevented):

Feature Fatty acid synthesis Fatty acid β-oxidation
Location Cytosol Mitochondrial matrix
Carrier Acyl carrier protein (ACP) of FAS Coenzyme A
Carbon unit added/removed 2-C as malonyl-CoA (3-C donor, loses CO₂) 2-C as acetyl-CoA
Reducing/oxidising equivalent NADPH (uses) FAD + NAD⁺ (generates FADH₂, NADH)
Key vitamin Biotin (B7) for ACC; pantothenate in ACP Riboflavin (FAD), niacin (NAD⁺)
Activated/inhibited state Well-fed, high insulin Fasting, high glucagon
Committed/regulatory step Acetyl-CoA carboxylase (ACC) Carnitine CPT-1 (entry)
Inhibitor signal Palmitoyl-CoA, glucagon (↓) Malonyl-CoA inhibits CPT-1

High-yield: The single most-tested reciprocal control fact — malonyl-CoA, the first committed product of synthesis, inhibits CPT-1 and thus blocks β-oxidation. When you are making fat, you cannot burn it.


Part 1 — De novo fatty acid synthesis (lipogenesis)

Where the substrate comes from: the citrate shuttle

Acetyl-CoA is generated in the mitochondrion but FAS is cytosolic, and acetyl-CoA cannot cross the inner mitochondrial membrane. It is exported as citrate.

Flow: Acetyl-CoA + OAA → citrate (citrate synthase) → citrate exits via tricarboxylate carrier → in cytosol, ATP-citrate lyase cleaves citrate → acetyl-CoA + OAA → OAA → malate (MDH) → malate → pyruvate by malic enzyme, generating NADPH.

High-yield: The citrate shuttle simultaneously delivers acetyl-CoA and contributes NADPH (via malic enzyme). The other major NADPH source for lipogenesis is the HMP (pentose phosphate) shunt.

Step 1 — Acetyl-CoA carboxylase (ACC): the committed, rate-limiting step

Acetyl-CoA + CO₂ + ATP → malonyl-CoA (3 carbons)

  • Cofactor: biotin (carboxylation enzyme — remember pyruvate carboxylase, propionyl-CoA carboxylase, ACC all use biotin).
  • ACC exists as inactive protomers and active polymers.

Regulation of ACC (the regulatory heart of the pathway):

Activator Inhibitor
Citrate (allosteric → polymerisation) Palmitoyl-CoA (end-product, depolymerises)
Insulin (dephosphorylation → active) Glucagon/adrenaline (phosphorylation → inactive)
AMPK phosphorylates and inactivates ACC

High-yield: Insulin activates ACC by dephosphorylation; glucagon and AMPK inactivate it by phosphorylation. Citrate is the allosteric activator; palmitoyl-CoA is the feedback inhibitor.

Step 2 — The fatty acid synthase (FAS) complex

In humans, FAS is a single multifunctional dimeric polypeptide with 7 catalytic activities + ACP. Each monomer carries a phosphopantetheine arm (derived from pantothenic acid / vitamin B5) on ACP, plus a cysteine –SH on the condensing enzyme (ketoacyl synthase).

The repeating elongation cycle adds 2 carbons each turn — mnemonic "Can Anyone Really Drive A Car" is not standard; use the functional sequence:

Condensation → Reduction → Dehydration → Reduction

  1. Condensation (β-ketoacyl synthase): acetyl (on Cys-SH) + malonyl (on ACP) → 4-C β-ketoacyl-ACP + CO₂ released.
  2. Reduction (β-ketoacyl reductase): uses NADPH → β-hydroxyacyl-ACP.
  3. Dehydration (dehydratase): → enoyl-ACP (trans double bond).
  4. Reduction (enoyl reductase): uses NADPH → saturated acyl-ACP.

After 7 cycles, palmitate (C16, saturated) is released by thioesterase.

Stoichiometry for palmitate:

Acetyl-CoA + 7 Malonyl-CoA + 14 NADPH + 14 H⁺ → Palmitate + 7 CO₂ + 8 CoA + 14 NADP⁺ + 6 H₂O

Including the 7 ACC reactions: 8 acetyl-CoA + 7 ATP + 14 NADPH → 1 palmitate.

High-yield: Palmitate (16C) is the sole product of the cytosolic FAS complex. Elongation beyond C16 and desaturation occur in the smooth endoplasmic reticulum (microsomal system, uses malonyl-CoA + NADPH). Mitochondria perform minor elongation using acetyl-CoA + NADPH/NADH.

Desaturation

Microsomal Δ⁹, Δ⁶, Δ⁵, Δ⁴ desaturases introduce double bonds, requiring O₂, NADH, cytochrome b₅. Humans cannot desaturate beyond C9 toward the methyl end → cannot make linoleic (ω-6) and α-linolenic (ω-3) acids → these are essential fatty acids. Arachidonic acid becomes essential only if linoleic acid is deficient.


Part 2 — The carnitine shuttle (entry into β-oxidation)

Long-chain fatty acyl-CoA cannot cross the inner mitochondrial membrane. The carnitine shuttle is the gateway and a favourite exam target.

Flow:

  1. FA activated in cytosol → acyl-CoA by acyl-CoA synthetase (thiokinase) on outer mitochondrial membrane; costs 2 high-energy bonds (ATP → AMP + 2 Pi).
  2. CPT-1 (carnitine palmitoyltransferase-1) on outer membrane swaps CoA for carnitine → acylcarnitine. Rate-limiting step; inhibited by malonyl-CoA.
  3. Carnitine-acylcarnitine translocase (CACT) carries acylcarnitine in, carnitine out.
  4. CPT-2 on inner membrane regenerates acyl-CoA in the matrix.

High-yield: Carnitine is synthesised from lysine + methionine in liver/kidney (needs vitamin C). CPT-1 deficiency → hypoketotic hypoglycaemia, hepatomegaly, normal/low muscle carnitine. CPT-2 deficiency (commonest) → adult exercise-induced myopathy, rhabdomyolysis, myoglobinuria. Primary carnitine deficiency = defect in OCTN2 carnitine transporter → cardiomyopathy.

Note: Short- and medium-chain fatty acids enter mitochondria independently of carnitine.


Part 3 — β-Oxidation

Occurs in the mitochondrial matrix. Each cycle shortens the chain by 2 carbons and follows four steps — mnemonic "Oxidation, Hydration, Oxidation, Cleavage" or the enzyme order:

Acyl-CoA → (1) FAD oxidation → (2) hydration → (3) NAD⁺ oxidation → (4) thiolytic cleavage → Acetyl-CoA + acyl-CoA (n–2)

Step Enzyme Reaction Product / equivalent
1 Acyl-CoA dehydrogenase (chain-length specific: VLCAD, LCAD, MCAD, SCAD) Oxidation FADH₂ (→1.5 ATP)
2 Enoyl-CoA hydratase Hydration of trans double bond 3-hydroxyacyl-CoA
3 3-hydroxyacyl-CoA dehydrogenase Oxidation NADH (→2.5 ATP)
4 β-ketothiolase (thiolase) Thiolytic cleavage Acetyl-CoA + shortened acyl-CoA

The first step's FADH₂ feeds electrons via ETF (electron-transferring flavoprotein) → ETF-QO → ubiquinone.

ATP yield — the calculation you must be able to do fast

For palmitate (C16, fully saturated), modern P/O ratios (NADH = 2.5, FADH₂ = 1.5):

  • Cycles = (16/2) − 1 = 7 cycles → 7 FADH₂ + 7 NADH
  • Acetyl-CoA produced = 16/2 = 8, each via TCA = 10 ATP → 80
  • From β-oxidation: 7 × (1.5 + 2.5) = 28
  • Gross = 80 + 28 = 108
  • Subtract 2 for activation (ATP→AMP) → Net = 106 ATP

High-yield: Palmitate net = 106 ATP (new values) or 129 ATP (old values: NADH=3, FADH₂=2). Know the formula: for a saturated FA with n carbons, acetyl-CoA = n/2, cycles = (n/2 − 1). Always subtract 2 for activation.

Odd-chain fatty acid oxidation

Final cycle yields acetyl-CoA + propionyl-CoA (3C).

Flow: Propionyl-CoA → (propionyl-CoA carboxylase, biotin) → D-methylmalonyl-CoA → (racemase) → L-methylmalonyl-CoA → (methylmalonyl-CoA mutase, vitamin B12 / adenosylcobalamin) → succinyl-CoA → TCA / gluconeogenesis.

High-yield: This is the only route by which fatty acids contribute to gluconeogenesis (via the propionyl-CoA → succinyl-CoA anaplerotic carbon). Vitamin B12 deficiency → ↑ methylmalonic acid (methylmalonic aciduria); a classic distinguishing lab from folate deficiency. Branched-chain (phytanic acid) and isoleucine/valine/methionine catabolism also produce propionyl-CoA.

Unsaturated fatty acid oxidation

Requires two extra enzymes:

  • Enoyl-CoA isomerase — converts cis-Δ³ to trans-Δ² double bonds (for mono/poly-unsaturated).
  • 2,4-dienoyl-CoA reductase (uses NADPH) — for polyunsaturated FAs.

Each pre-existing double bond means one fewer FADH₂-generating step → slightly less ATP than the equivalent saturated FA.

Other oxidation routes (rapid)

  • α-oxidation (peroxisomes/ER): for branched-chain phytanic acid (β-carbon is blocked by methyl). Defect → Refsum disease (retinitis pigmentosa, cerebellar ataxia, peripheral neuropathy, ichthyosis).
  • ω-oxidation (microsomal): produces dicarboxylic acids; minor, increases in MCAD deficiency.
  • Peroxisomal β-oxidation: handles very-long-chain FA (VLCFA); uses FAD → H₂O₂ (not ATP). Defect in transporter → X-linked adrenoleukodystrophy (ALD) with raised VLCFA; Zellweger syndrome = absent peroxisomes.

Part 4 — Ketone bodies (linked downstream)

Excess acetyl-CoA from hepatic β-oxidation during fasting/diabetes → ketogenesis in liver mitochondria.

Flow: 2 acetyl-CoA → acetoacetyl-CoA → (HMG-CoA synthase, rate-limiting) HMG-CoA → (HMG-CoA lyase) acetoacetateβ-hydroxybutyrate (major in blood) and spontaneous → acetone.

High-yield: Liver makes but cannot use ketone bodies — it lacks thiophorase (succinyl-CoA acetoacetyl-CoA transferase / SCOT). Extrahepatic tissues (brain, muscle, heart) use them. β-hydroxybutyrate:acetoacetate ratio rises in severe ketoacidosis; nitroprusside dipsticks detect acetoacetate/acetone, NOT β-hydroxybutyrate — hence ketosis may be underestimated early in DKA.


Inborn errors — MCAD and friends

MCAD deficiency (medium-chain acyl-CoA dehydrogenase)

The commonest inherited fatty-acid oxidation disorder; autosomal recessive; common ACADM gene mutation K304E (985A>G).

  • Presents at 3 months–2 years after a fasting/illness trigger (prolonged fast, intercurrent infection).
  • Hypoketotic hypoglycaemia (cannot oxidise FA → no acetyl-CoA → no ketones, and gluconeogenesis substrate falls), lethargy, vomiting, seizures, coma; may mimic SIDS / Reye-like picture.
  • Lab: dicarboxylic aciduria (C6–C10), low/absent ketones, raised C8 (octanoyl) acylcarnitine on tandem mass spectrometry (newborn screening marker).
  • Management: avoid fasting, frequent feeds, IV dextrose during illness; generally good prognosis once recognised.

High-yield: Hypoketotic hypoglycaemia + dicarboxylic aciduria + raised C8-acylcarnitine = MCAD deficiency. Contrast with hyperketotic hypoglycaemia of glycogen storage / ketotic states. Treatment is dietary: never fast.

Disorder Enzyme/defect Hallmark
MCAD deficiency Medium-chain acyl-CoA DH (ACADM) Hypoketotic hypoglycaemia, ↑C8, dicarboxylic aciduria
CPT-1 deficiency Carnitine palmitoyltransferase-1 Hypoketotic hypoglycaemia, hepatomegaly, ↑ carnitine
CPT-2 deficiency CPT-2 (commonest carnitine defect) Adult exertional myopathy, rhabdomyolysis
Primary carnitine deficiency OCTN2 transporter Cardiomyopathy, low plasma carnitine
Jamaican vomiting sickness Hypoglycin A (unripe ackee fruit) inhibits acyl-CoA DH Hypoglycaemia, vomiting
Refsum disease Phytanoyl-CoA hydroxylase (α-oxidation) Phytanic acid ↑, retinitis pigmentosa
X-linked ALD Peroxisomal VLCFA transporter (ABCD1) ↑ VLCFA, adrenal + CNS demyelination

Key differentials & cross-links

  • Hypoglycaemia + low ketones → fatty-acid oxidation defect (MCAD, CPT) or hyperinsulinism. Hypoglycaemia + high ketones → glycogen storage / ketotic hypoglycaemia / GH-cortisol deficiency.
  • Methylmalonic aciduria → B12 deficiency or mutase defect (odd-chain FA / propionate pathway).
  • Biotin is shared by ACC, pyruvate carboxylase, propionyl-CoA carboxylase, methylcrotonyl-CoA carboxylase — multiple carboxylase deficiency presents with combined metabolic acidosis, alopecia, rash.

Recently asked / exam angle

  • "Which inhibits CPT-1?" → Malonyl-CoA (most repeated single fact).
  • "Rate-limiting enzyme of fatty acid synthesis?" → Acetyl-CoA carboxylase; cofactor biotin.
  • "NADPH for lipogenesis comes from?" → HMP shunt + malic enzyme.
  • "Number of NADPH used to make palmitate?" → 14.
  • "Site of fatty acid synthesis vs oxidation?" → cytosol vs mitochondrial matrix.
  • "Net ATP from complete oxidation of palmitate?" → 106 (or 129 old).
  • "Enzyme needing B12 in odd-chain oxidation?" → methylmalonyl-CoA mutase.
  • "Commonest FA oxidation disorder / hypoketotic hypoglycaemia in infant?" → MCAD deficiency (↑C8).
  • "Enzyme liver lacks for ketone utilisation?" → thiophorase (SCOT).
  • "Unripe ackee fruit toxin?" → hypoglycin A inhibiting acyl-CoA dehydrogenase.
  • Image/diagram-based: identifying the 4-step β-oxidation spiral or citrate shuttle.

Rapid revision

  1. Synthesis = cytosol, NADPH, ACP, makes palmitate (C16) only; oxidation = matrix, FAD/NAD⁺, CoA.
  2. ACC (biotin) is rate-limiting for synthesis: citrate activates, palmitoyl-CoA + glucagon + AMPK inhibit; insulin activates by dephosphorylation.
  3. Malonyl-CoA is the 2-C donor for synthesis AND the inhibitor of CPT-1 — the reciprocal switch.
  4. Human FAS = one multifunctional dimer, 7 activities + ACP (phosphopantetheine from vitamin B5).
  5. Citrate shuttle exports acetyl-CoA and yields NADPH via malic enzyme; HMP shunt is the other NADPH source.
  6. 14 NADPH + 7 ATP + 8 acetyl-CoA → palmitate.
  7. Carnitine shuttle: CPT-1 (outer, rate-limiting) → CACT → CPT-2 (inner); short/medium-chain FA bypass carnitine.
  8. β-oxidation spiral: oxidation (FADH₂) → hydration → oxidation (NADH) → thiolysis (acetyl-CoA).
  9. Palmitate complete oxidation = net 106 ATP (subtract 2 for activation).
  10. Odd-chain → propionyl-CoA → (B12 mutase) → succinyl-CoA: only FA route feeding gluconeogenesis; B12 deficiency → methylmalonic aciduria.
  11. MCAD deficiency: hypoketotic hypoglycaemia + dicarboxylic aciduria + ↑C8-acylcarnitine; treat by avoiding fasting.
  12. Liver makes ketones but cannot use them (no thiophorase); β-hydroxybutyrate is the major blood ketone but is missed by nitroprusside sticks.